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Hoffmann, R. A wiki for the life sciences where authorship matters. Nature Genetics (2008)
 

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Salen complexes with bulky substituents as useful tools for biomimetic phenol oxidation research.

The catalytic properties of bulky water-soluble Co-, Cu-, Fe- and Mn-salen complexes in the oxidation of phenolic lignin model compounds have been studied in aqueous water--dioxane solutions (pH 3--10). Mn catalysts were found to oxidize coniferyl alcohol in a same reaction time as horseradish peroxidase (HRP) enzyme and Mn and Co catalysts showed different regioselectivity suggesting a different substrate to catalyst interaction in the oxidative coupling. When the oxidation of material more relevant to plant polyphenolics was studied, the results indicated that the complexes catalyze one- and two-electron oxidations depending on the bulk of the substrate.[1]

References

  1. Salen complexes with bulky substituents as useful tools for biomimetic phenol oxidation research. Haikarainen, A., Sipilä, J., Pietikäinen, P., Pajunen, A., Mutikainen, I. Bioorg. Med. Chem. (2001) [Pubmed]
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